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Review: Tip-based vibrational spectroscopy for nanoscale analysis of emerging energy materials

Amun JARZEMBSKI, Cedric SHASKEY, Keunhan PARK

Frontiers in Energy 2018, Volume 12, Issue 1,   Pages 43-71 doi: 10.1007/s11708-018-0524-8

Abstract: the AFM tip as a nanoscopic tool to extract spatially resolved electronic or molecular vibrational resonancelight by electrons or individual functional groups within molecules leads to changes in the sample’s thermalFor example, photothermal induced resonance (PTIR) spectroscopy methods measure a sample’s local thermalTherefore, they use the AFM tip as a thermal detector to directly relate absorbed IR light to the thermalMore recently, photo-induced force microscopy (PiFM) has been developed to measure the change of the

Keywords： vibrational spectroscopy     atomic force microscopy     photo-thermal induced resonance     scanning near-fieldoptical microscopy     tip-enhanced Raman spectroscopy     photo-induced force microscopy     molecular resonances    

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Solar fuel from photo-thermal catalytic reactions with spectrum-selectivity: a review

Sanli TANG, Jie SUN, Hui HONG, Qibin LIU

Frontiers in Energy 2017, Volume 11, Issue 4,   Pages 437-451 doi: 10.1007/s11708-017-0509-z

Abstract: The synergy of photo and thermal effects leads to a new approach to higher solar fuel production underThis paper reviews different approaches for solar fuel production from spectrum-selective photo-thermalreview begins with the meaning of synergetic effects, and the mechanisms of spectrum-selectivity and photo-thermalA discussion is finally presented concerning future development of photo-thermal catalytic reactions

Keywords： photo-thermal catalysis     spectrum-selectivity     solar fuel     full-spectrum    

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Hypoxia-induced activity loss of a photo-responsive microtubule inhibitor azobenzene combretastatin A4

Yang An, Chao Chen, Jundong Zhu, Pankaj Dwivedi, Yanjun Zhao, Zheng Wang

Frontiers of Chemical Science and Engineering 2020, Volume 14, Issue 5,   Pages 880-888 doi: 10.1007/s11705-019-1864-6

Abstract: The conformation-dependent activity of azobenzene combretastatin A4 (Azo-CA4) provides a unique approach to reduce the side-effects of chemotherapy, due to the light-triggered conformation transition of its azobenzene moiety. Under hypoxic tumor microenvironment, however, the high expression of azoreductase can reduce azobenzene to aniline. It was postulated that the Azo-CA4 might be degraded under hypoxia, resulting in the decrease of its anti-tumor activity. The aim of this study was to verify such hypothesis in HeLa cells . The quantitative drug concentration analysis shows the ratiometric formation of degradation end-products, confirming the bioreduction of Azo-CA4. The tubulin staining study indicates that Azo-CA4 loses the potency of switching off microtubule dynamics under hypoxia. Furthermore, the cell cycle analysis shows that the ability of Azo-CA4 to induce mitotic arrest is lost at low oxygen content. Therefore, the cytotoxicity of Azo-CA4 is compromised under hypoxia. In contrast, combretastatin A4 as a positive control maintains the potency to inhibit tubulin polymerization and break down the nuclei irrespective of light irradiation and oxygen level. This work highlights the influence of hypoxic tumor microenvironment on the anti-tumor potency of Azo-CA4, which should be considered during the early stage of designing translational Azo-CA4 delivery systems.

Keywords： hypoxia     microtubule inhibitor     drug delivery     azo-combretastatin A4     photo-responsive    

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Photo-induced surface frustrated Lewis pairs for promoted photocatalytic decomposition of perfluorooctanoic

Frontiers of Environmental Science & Engineering 2023, Volume 17, Issue 1, doi: 10.1007/s11783-023-1603-6

Abstract:

● Terminal carboxylate group activation is PFOA degradation’s rate-limiting step.

Keywords： Heterogeneous photocatalysis     Surface frustrated Lewis pairs     Perfluorooctanoic acid     Defluorination efficiency     Environmental remediation    

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Experimental and computational assessment of 1,4-Dioxane degradation in a photo-Fenton reactive ceramic

Frontiers of Environmental Science & Engineering 2021, Volume 15, Issue 5, doi: 10.1007/s11783-020-1341-y

Abstract:

• 1,4-Dioxane was degraded via the photo-Fenton reactive membrane filtration

Keywords： Photo-Fenton     Ceramic membrane     1     4-Dioxane     Goethite    

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Selective reduction of NO by photo-SCR with ammonia in an annular fixed-film photoreactor

YiangChen CHOU, Young KU

Frontiers of Environmental Science & Engineering 2012, Volume 6, Issue 2,   Pages 149-155 doi: 10.1007/s11783-010-0296-9

Abstract: Gaseous NO was photocatalytically reduced at room temperature by photo-assisted selective catalytic reduction(photo-SCR) with ammonia over TiO in this study.The kinetic model proposed in this study can be used to reasonably describe the reaction mechanism of photo-SCR

Keywords： photo-SCR     photocatalysis     NO reduction     Eley-Rideal model    

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Lignin-based electrospun nanofiber membrane decorated with photo-Fenton Ag@MIF-100(Fe) heterojunctions

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 7,   Pages 930-941 doi: 10.1007/s11705-023-2309-9

Abstract: /i> seeding method to fabricate a lignin-based electrospun nanofiber membrane (LENM) decorated with photo-Fentonwithin 30 min under illumination, which is attributed to a synergy of dye adsorption/enrichment and photo-FentonTherefore, the lignin-based photo-Fenton hybrid membrane can lay the foundation for the preparation and

Keywords： lignin     electrospinning     heterojunctions     photo-Fenton catalysis     wastewater remediation    

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Synthesis, spectroscopic, and electrochemical properties of two dyads consisted of tetrathiafulvalene and carbazole

Guoqiao LAI, Yibo LIU, Meijiang LI, Yongjia SHEN

Frontiers of Chemical Science and Engineering 2009, Volume 3, Issue 2,   Pages 192-195 doi: 10.1007/s11705-009-0015-x

Abstract: Compared with carbazole, their fluorescence was strongly quenched, which implied that a photo induced

Keywords： donor-σ-acceptor molecule     intramolecular charge transfer interaction     photo induced electron transfer    

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Highly selective detection of copper(II) by a “ligand-free” conjugated copolymer in nucleophilic solvents

Weixing Deng, Pengfei Sun, Quli Fan, Lei Zhang, Tsuyoshi Minami

Frontiers of Chemical Science and Engineering 2020, Volume 14, Issue 1,   Pages 105-111 doi: 10.1007/s11705-019-1791-6

Abstract: observed at low temperature suggests that the quenching and reducing mechanism is most probably due to a photo-induced

Keywords： ligand-free     fluorescent chemosensor     copper     photo-induced electron transfer    

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Multi-harmonic forced vibration and resonance of simple beams to moving vehicles

Frontiers of Structural and Civil Engineering   Pages 981-993 doi: 10.1007/s11709-023-0979-5

Abstract: This study modeled the moving-vehicle-induced forcing excitation on a single-span prismatic bridge asof a linear elastic simple Euler–Bernoulli beam, and investigated the forced modal oscillation and resonanceThe analysis revealed that a moving load induces high-harmonic forced resonance amplification when theTo verify the occurrence of high-harmonic forced resonance, numerical tests were conducted on single-spanThe forced resonance amplification characteristics of the fundamental mode for beam response estimation

Keywords： forced vibration     linear Euler beam     moving load     harmonic structure     frequency modulation     end restraints    

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Sectional model test study on vortex-excited resonance of vehicle-bridge system of Shanghai Bridge over

Li ZHOU, Yaojun GE

Frontiers of Structural and Civil Engineering 2009, Volume 3, Issue 1,   Pages 67-72 doi: 10.1007/s11709-009-0007-4

Abstract: It is necessary to study how vehicles influence the vortex-excited resonance of vehicle-bridge systems, because lock-in wind speed is low and vortex-excited resonance is sensitive to any change in the mainBased on the Shanghai Bridge over the Yangtse River, the vortex-excited resonance of a 1∶60 scale sectionalThe result indicates that: 1) for the bridge with vehicles, the vertical vortex-excited resonance isTherefore, the influence of vehicles on vortex-excited resonance performance of vehicle-bridge systems

Keywords： vehicle-bridge system     sectional mode     vortex-excited resonance     wind tunnel test     mode shape correction    

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A method of determining flame radiation fraction induced by interaction burning of tri-symmetric propane

Jie JI, Junrui DUAN, Huaxian WAN

Frontiers in Energy 2022, Volume 16, Issue 6,   Pages 1017-1026 doi: 10.1007/s11708-020-0716-x

Abstract: almost identical to a single fire; for merging flames ( / ≤0.368), based on the relationship between thermal

Keywords： flame interaction     air entrainment     flame height     multi-point source model     thermal radiation    

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Discovery of the mechanisms of acupuncture in the treatment of migraine based on functional magnetic resonance

Frontiers of Medicine   Pages 993-1005 doi: 10.1007/s11684-023-0989-7

Abstract: The functional magnetic resonance imaging (fMRI) data were analyzed for investigating brain changes induced

Keywords： acupuncture     migraine     fMRI     metabolome     proteome    

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Extended stochastic resonance (SR) and its applications in weak mechanical signal processing

Niaoqing HU, Min CHEN, Guojun QIN, Lurui XIA, Zhongyin PAN, Zhanhui FENG,

Frontiers of Mechanical Engineering 2009, Volume 4, Issue 4,   Pages 450-461 doi: 10.1007/s11465-009-0072-3

Abstract: This paper presents a method based on stochastic resonance (SR) to detect weak fault signal.

Keywords： extended stochastic resonance (SR)     stability analysis of SR     scale transform     weak signal detection     incipient    

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Cyanobacterial photo-driven mixotrophic metabolism and its advantages for biosynthesis

Ni Wan,Mary Abernathy,Joseph Kuo-Hsiang Tang,Yinjie J. Tang,Le You

Frontiers of Chemical Science and Engineering 2015, Volume 9, Issue 3,   Pages 308-316 doi: 10.1007/s11705-015-1521-7

Abstract: The photo-fermentations show enhanced photosynthesis, while CO loss from organic substrate degradationThe use of cyanobacteria as “green ” could be a promising route to develop robust photo-biorefineries

Keywords： CO2 mass transfer     N2 fixation     photosystem     RuBisCO     the TCA cycle    

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Title Author Date Type Operation

Review: Tip-based vibrational spectroscopy for nanoscale analysis of emerging energy materials

Amun JARZEMBSKI, Cedric SHASKEY, Keunhan PARK

Journal Article

Solar fuel from photo-thermal catalytic reactions with spectrum-selectivity: a review

Sanli TANG, Jie SUN, Hui HONG, Qibin LIU

Journal Article

Hypoxia-induced activity loss of a photo-responsive microtubule inhibitor azobenzene combretastatin A4

Yang An, Chao Chen, Jundong Zhu, Pankaj Dwivedi, Yanjun Zhao, Zheng Wang

Journal Article

Photo-induced surface frustrated Lewis pairs for promoted photocatalytic decomposition of perfluorooctanoic

Journal Article

Experimental and computational assessment of 1,4-Dioxane degradation in a photo-Fenton reactive ceramic

Journal Article

Selective reduction of NO by photo-SCR with ammonia in an annular fixed-film photoreactor

YiangChen CHOU, Young KU

Journal Article

Lignin-based electrospun nanofiber membrane decorated with photo-Fenton Ag@MIF-100(Fe) heterojunctions

Journal Article

Synthesis, spectroscopic, and electrochemical properties of two dyads consisted of tetrathiafulvalene and carbazole

Guoqiao LAI, Yibo LIU, Meijiang LI, Yongjia SHEN

Journal Article

Highly selective detection of copper(II) by a “ligand-free” conjugated copolymer in nucleophilic solvents

Weixing Deng, Pengfei Sun, Quli Fan, Lei Zhang, Tsuyoshi Minami

Journal Article

Multi-harmonic forced vibration and resonance of simple beams to moving vehicles

Journal Article

Sectional model test study on vortex-excited resonance of vehicle-bridge system of Shanghai Bridge over

Li ZHOU, Yaojun GE

Journal Article

A method of determining flame radiation fraction induced by interaction burning of tri-symmetric propane

Jie JI, Junrui DUAN, Huaxian WAN

Journal Article

Discovery of the mechanisms of acupuncture in the treatment of migraine based on functional magnetic resonance

Journal Article

Extended stochastic resonance (SR) and its applications in weak mechanical signal processing

Niaoqing HU, Min CHEN, Guojun QIN, Lurui XIA, Zhongyin PAN, Zhanhui FENG,

Journal Article

Cyanobacterial photo-driven mixotrophic metabolism and its advantages for biosynthesis

Ni Wan,Mary Abernathy,Joseph Kuo-Hsiang Tang,Yinjie J. Tang,Le You

Journal Article